By Allen J. Bard, Israel Rubinstein
ISBN-10: 082479379X
ISBN-13: 9780824793791
This paintings offers finished experiences on fresh advancements and functions of well-established suggestions within the box of contemporary electro- and electodynamical chemistry. It provides discussions of proven suggestions and of components nonetheless less than research, and covers peripherally similar components, together with the kinematics and mechanics of electrode reactions, that may be utilized to electrochemical difficulties.
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Additional info for Electroanalytical chemistry: a series of advances
Example text
The reaction zone is at the outer edge of the depletion zone, under the conditions of the plot in Fig. 1. Here, incoming A and outgoing D encounter to form B and C. Equilibrium (16), under the conditions mentioned, is shifted far to the right. 3. These problems are worse if reactions of an order higher than unity are considered. Then, the kinetic term is no longer linear in the concentrations to be calculated. The entire differential equation system becomes nonlinear. 4. Nonlinearity may also be present in the boundary conditions, for example, if the concentrations at the electrode surface (x = 0) are determined by adsorption isotherms.
The concentrations at discrete points in space after a discrete time step t + Dt are calculated from the concentrations at these points before the time step (t; explicit FD [EFD]; see Fig. 1 for a graphical representation) or they are expressed by the c before and after the time step (implicit or semiimplicit FD) [44]. , [7]) have been formulated, and some of these are discussed in this review. Boxes [2] and points [7] have been chosen as the elementary spatial discretization units. In this review, the term space element will be employed to designate both of these approaches, and these elements will be indexed by i.
Chapters vary in length and subject area. Some are reviews of recent developments and applications of well-established techniques, whereas others contain discussion of the background and problems in areas still being investigated extensively and in which many statements may still be tentative. Finally, chapters on techniques generally outside the scope of electroanalytical chemistry, but which can be applied fruitfully to electrochemical problems, are included. Electroanalytical chemists and others are concerned not only with the application of new and classical techniques to analytical problems, but also with the fundamental theoretical principles upon which these techniques are based.
Electroanalytical chemistry: a series of advances by Allen J. Bard, Israel Rubinstein
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